Abstract The accurate theoretical description of materials with strongly correlated electrons is a formidable challenge in condensed matter physics and computational chemistry. Dynamical Mean Field Theory (DMFT) is a successful approach that predicts behaviors of such systems by incorporating some of the correlated behavior using an impurity model, but it is limited by the need to calculate the impurity Green’s function. This work proposes a framework for DMFT calculations on quantum computers, focusing on near-term applications. It leverages the structure of the impurity problem, combining a low-rank Gaussian subspace representation of the ground state and a compressed, short-depth quantum circuit that joins state preparation with time evolution to compute Green’s functions. We demonstrate the convergence of the DMFT algorithm using the Gaussian subspace in a noise-free setting, and show the hardware viability of circuit compression by extracting the impurity Green’s function on IBM quantum processors for a single impurity coupled to three bath orbitals (8 qubits, 1 ancilla). We discuss potential paths toward realizing this quantum computing use case in materials science. Acknowledgements We acknowledge helpful discussions with Steve Johnston. N.H. and A.F.K. were supported by the U.S. National Science Foundation under Grant No. DMR-1752713. E.K., D.C., and R.V.B. were supported by the U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231 through the Office of Advanced Scientific Computing Research Accelerated Research for Quantum Computing Program. W.A.dJ. acknowledges support from the "Embedding Quantum Computing into Manybody Frameworks for Strongly Correlated Molecular and Materials Systems" project, by the U.S. DOE, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. Ethics declarations Competing interests The authors declare no competing interests. Additional information Publisher’s note Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations. Supplementary information Rights and permissions Open Access